Marcus Brody (archive footage) (uncredited)
Self (archive footage)
Selsdon Mowbray / The Burglar
Father LeBlanc
George Smiley
Howler
Headmaster
William Filmore
Thomas Wilkins
James O'Hannon
Marcus Brody
Colonel Grayson
Fulbert
Inspector Basil Crisp
Old Geraint
Howard
Dr. Barry
Sir Henry 'Jock' Delves Broughton
Salter
Victor
Vernon Bayliss
Col. Phelps
George Parker
Philip Neville
Mr. Emerson
Dr. Savary
Count de Noilly
Dr. Swaby
Elliott Templeton
Dr. Mortimer
Coleman
Sir Ralph Skelton
Tom Bates
The Bishop of London
Tom Bates
Dr. Marcus Brody
Parker (segment "An Englishman's Home")
Jack Hill
Raglan Thistle
Charles Seymour
Stefan Vognic
Alan Quine
Donald Skinner
Colonel Pulleine
William Leigh
Cowslip (voice)
Sidney Beynon
Stapleton
ex-Detective Chief Superintendent Jupp
English Delegate
RAF meteorologist officer
The Signalman
Admiral Canaris
Will Scarlet
Henry Beddows
John Grey
John Petapiece
Dr. Frank Henson
Sir Emmanuel Whitbread
Robert Murray
Nils Krogstad
Diltant (segment 5 "Drawn and Quartered")
malcom De Vere
Tom Lewis
Charles Hillyer (segment 1 "Method for Murder")
Emmanuel Whitbread
Peter NIss
Captain Hornsby
Dr. Yevgeny Dorn
Vance Fowler
Gerald
Mr. George Beauchamp
George Devlin
Inspector Barrada
Pond-Jones
The Abortionist
Larkin
Captain Tabasco
Herbert
Charlie Prince
Montague Corry
Oliver Larker
The Writer
Sir Robert Morton
Edgar Norton
Arthur Grimble
Fl. Lt. McKenzie
Martin Blake
Sergeant Corcoran
The Chimney Sweep (voice)
Morell
Michael Gregory
John Lemley
Christopher Ridgefield
Oswald Morfrey